Journal2017دسترسی آزاد

Synthesis of novel magnetic nanoparticles with urea or urethane moieties: Applications as catalysts in the Strecker synthesis of α‐aminonitriles

Saeed Baghery, Mohammad Ali Zolfigol, Romana Schirhagl, Masoumeh Hasani, Marc C. A. Stuart, Andreas Nagl

Applied Organometallic Chemistry Vol. 31, No. 12

چکیده

Four novel magnetic nanoparticle catalysts with urea or urethane moieties are reported. The silica‐coated magnetic nanoparticles were simply functionalized via addition of 3‐(triethoxysilyl)propylisocyanate (TESPIC), amine or amino alcohol. TESPIC with dual labile functional groups was used as a suitable precursor for the synthesis of urethane‐based catalysts. The newly synthesized catalysts were fully characterized using a variety of techniques. These functionalized magnetic nanoparticles were used as reusable catalysts in the Strecker synthesis of α‐aminonitrile derivatives under solvent‐free conditions at 50 °C.

موضوعات و کلیدواژه‌ها

Chemical Synthesis and ReactionsSulfur-Based Synthesis TechniquesSynthesis of Indole DerivativesChemistryStrecker amino acid synthesisCatalysisNanoparticleUreaMagnetic nanoparticlesAmine gas treatingSolventAlcoholOrganic chemistryCombinatorial chemistryNanotechnologyEnantioselective synthesisMaterials science

ارجاع علمی

Saeed Baghery, Mohammad Ali Zolfigol, Romana Schirhagl, Masoumeh Hasani, Marc C. A. Stuart, Andreas Nagl. “Synthesis of novel magnetic nanoparticles with urea or urethane moieties: Applications as catalysts in the Strecker synthesis of α‐aminonitriles.” Applied Organometallic Chemistry, 2017. https://doi.org/10.1002/aoc.3883